Energetics of stacking boundaries on the {0001} surfaces of silicon carbide.

MJ Rutter, V Heine, J Phys Cond Matt (1997) vol 9 pg 8213

Abstract

Silicon carbide often grows in the cubic phase under conditions where this is not the most stable phase. Ab initio calculations are presented which determine the energy of a stacking reversal at the (0001) and (000$\bar{1}$) surfaces of silicon carbide, and thus whether the cubic form is preferred in the vicinity of a free surface. In these calculations the surfaces are not reconstructed but hydrogen terminated, and care is taken to eliminate the spurious dipole-dipole interaction caused by the imposition of periodic boundary conditions, and also in estimating the amount of residual ionic relaxation. These calculations do show a clear distinction of 13 meV per surface pair between between the silicon and carbon surfaces, although the results are not in complete agreement with experminent.

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